Skip to main content

Advertisement

Log in

Identification of the sources of metal (lead) contamination in drinking waters in north-eastern Tasmania using lead isotopic compositions.

  • Research Article
  • Published:
Environmental Science and Pollution Research Aims and scope Submit manuscript

Abstract

This study utilises a range of scientific approaches, including lead isotopic compositions, to differentiate unknown sources of ongoing lead contamination of a drinking water supply in north-eastern Tasmania, Australia. Drinking water lead concentrations are elevated above the Australian Drinking Water Guideline (10 μg/L), reaching 540 μg/L in the supply network. Water lead isotopic compositions from the town of Pioneer (208Pb/207Pb 2.406, 206Pb/207Pb 1.144 to 208Pb/207Pb 2.360, 206Pb/207Pb 1.094) and Ringarooma (208Pb/207Pb 2.398, 206Pb/207Pb 1.117) are markedly different from the local bedrock (208Pb/207Pb 2.496, 206Pb/207Pb 1.237). The data show that the lead in the local waters is sourced from a combination of dilapidated drinking water infrastructure, including lead jointed pipelines, end-of-life polyvinyl chloride pipes and household plumbing. Drinking water is being inadvertently contaminated by aging infrastructure, and it is an issue that warrants investigation to limit the burden of disease from lead exposure.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Subscribe and save

Springer+ Basic
€34.99 /Month
  • Get 10 units per month
  • Download Article/Chapter or eBook
  • 1 Unit = 1 Article or 1 Chapter
  • Cancel anytime
Subscribe now

Buy Now

Price includes VAT (Germany)

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6

Similar content being viewed by others

Explore related subjects

Discover the latest articles, news and stories from top researchers in related subjects.

References

  • ABS (Australian Bureau of Statistics) (2011) Census of population and housing basic community profile [online]. Available: http://www.censusdata.abs.gov.au/census_services/getproduct/census/2011/communityprofile/GL_TAS502?opendocument&navpos=230. Accessed 26 Sep 2014

  • Al-Malack MH (2001) Migration of lead from unplasticized polyvinyl chloride pipes. J Hazard Mater 82:263–274

    Article  CAS  Google Scholar 

  • Balazs C, Ray I (2014) The drinking water disparities framework: on the origins and persistence of inequalities in exposure. Am J Public Health 104:603–611

    Article  Google Scholar 

  • Beswick A (2012) Pioneer interurption to water supply—community information. Ben Lomond Water, Launceston

    Google Scholar 

  • Black LP, Everard JL, Mcclenaghan MP, Korsch RJ, Calver CR, Fioretti AM, Brown AV, Foudoulis C (2010) Controls on Devonian-Carboniferous magmatism in Tasmania, based on inherited zircon age patterns, Sr, Nd and Pb isotopes, and major and trace element geochemistry. Aust J Earth Sci 57:933–968

    Article  CAS  Google Scholar 

  • Cirarda FB (1998) Lead in drinking water in the Greater Bilbao Area (Basque Country, Spain). Food Addit Contam 15:575–579

    Article  CAS  Google Scholar 

  • Debenham AJ (1910) Frome Dam, Moorina, Tasmania. Paper read before the Sydney University Engineering Society

  • del Toral MA, Porter A, Schock MR (2013) Detection and evaluation of elevated lead release from service lines: a field study. Environ Sci Technol 47:9300–9307

    Article  Google Scholar 

  • DHHS (Tasmanian Department of Health and Human Services) (2014a) Royal george water quality update [online]. Department of Health and Human Services. Available: http://www.dhhs.tas.gov.au/peh/alerts/public_health_updates/royal_george. Accessed 15 May 2014

  • DHHS (Tasmanian Department of Health and Human Services) (2014b) Rosebery water alert [online]. Department of Health and Human Services. Available: http://www.dhhs.tas.gov.au/news/2013/rosebery_water_alert. Accessed 15 May 2014

  • Dickens DJ (1990) The Mount Cameron Water Race a century of operation [online]. Tasmanian Department of Resources and Energy. Division of Mines and Mineral Resources - Report 1990/15. http://www.mrt.tas.gov.au/mrtdoc/dominfo/download/UR1990_15/UR1990_15.pdf. Accessed 19 March 2015

  • Englert N, Höring H (1994) Lead concentration in tap-water and in blood of selected schoolchildren in Southern Saxonia. Toxicol Lett 72:325–331

    Article  CAS  Google Scholar 

  • Evans A (2013) National Measurement Institute, Inorganics Section, Method NT2.63: Determination of isotopic ratios in water and aqueous extracts by high resolution inductively coupled plasma mass spectometry. National Measurement Institute, Australian Government, North Ryde

    Google Scholar 

  • GHD (GHD Group) (2013a) Report for Ben Lomond Water—BLW drinking water quality options for small towns, 32/16667. Hobart

  • GHD (GHD Group) (2013b) Report for Ben Lomond Water—Winnaleah, Herrick, Pioneer and Gladstone full treatment water supply options, 32/10294. Hobart

  • Graham CMW, Andrew B, Gilmour WH, Michael RM, Gordon DM, Stuart JR, John W (1996) Is lead in tap water still a public health problem? An observational study in Glasgow. Br Med J 313:979

    Article  Google Scholar 

  • Gulson BL (1985) Shale-hosted lead-zinc deposits in northern Australia; lead isotope variations. Econ Geol 80:2001–2012

    Article  CAS  Google Scholar 

  • Gulson BL (1986) Lead isotopes in mineral exploration. Elsevier, USA

    Google Scholar 

  • Gulson BL, Law AJ, Korsch MJ, Mizon KJ (1994) Effect of plumbing systems on lead content of drinking water and contribution to lead body burden. Sci Total Environ 144:279–284

    Article  CAS  Google Scholar 

  • Harvey PJ, Taylor MP, Handley HK (In review) Widespread environmental contamination hazards in agricultural soils from the use of lead joints in above ground large-scale water supply pipelines. Water Air and Soil Pollution

  • Heathcote M (2009) History of plastic pipe systems in Australia—general technical information. Plastics Industry Pipe Association of Australia Limited

  • Hergt J, Chappell B, Mcculloch M, Mcdougall I, Chivas R (1989) Geochemical and isotopic constraints on the origin of the Jurassic Dolerites of Tasmania. J Petrol 30:840–883

    Article  Google Scholar 

  • Jane Wyatt C, Fimbres C, Romo L, Méndez RO, Grijalva M (1998) Incidence of heavy metal contamination in water supplies in Northern Mexico. Environ Res 76:114–119

    Article  Google Scholar 

  • Jaquet JB (1894) Geology of the Broken Hill Lode and Barrier Ranges Mineral Field, New South Wales. Department of Mines and Agriculture, Sydney

    Google Scholar 

  • Johri M, Chandra D, Subramanian SV, Sylvestre M-P, Pahwa S (2014) MDG 7c for safe drinking water in India: an illusive achievement. Lancet 383:1379

    Article  Google Scholar 

  • Knighton AD (1987) Tin mining and sediment supply to the Ringarooma River, Tasmania, 1875–1979. Aust Geogr Stud 25:83–97

    Article  Google Scholar 

  • Knighton AD (1989) River adjustment to changes in sediment load: the effects of tin mining on the Ringarooma River, Tasmania, 1875–1984. Earth Surf Process Landf 14:333–359

    Article  Google Scholar 

  • Knighton AD (1991) Channel bed adjustment along mine-affected rivers of northeast Tasmania. Geomorphology 4:205–219

    Article  Google Scholar 

  • Knighton AD (1999) The gravel–sand transition in a disturbed catchment. Geomorphology 27:325–341

    Article  Google Scholar 

  • Kristensen L, Taylor M, Morrison A (2015) Lead and zinc dust depositions from ore trains chracterised using lead isotopic compositions. Environ Sci Processes Impacts 17:631–637

  • Kristensen L, Taylor M, Odigie K, Hibdon S, Flegal A (2014) Lead isotopic compositions of ash sourced from Australian bushfires. Environ Pollut 190:159–165

    Article  CAS  Google Scholar 

  • Lanphear B, Dietrich K, Auinger P, Cox C (2000) Cognitive deficits associated with blood lead concentrations <10 microg/dL in US children and adolescents. Environ Health Perspect 115:521–529

    CAS  Google Scholar 

  • Lanphear B, Hornung R, Khoury J, Yolton K, Baghurst P, Bellinger D, Canfield R, Dietrich K, Bornschein R, Greene T, Rothenberg S, Needleman H, Schnass L, Wasserman L, Graziano J, Roberts R (2005) Low-level environmental lead exposure and children’s intellectual function: an international pooled analysis. Environ Health Perspect 113:894–899

    Article  CAS  Google Scholar 

  • Larsen MM, Blusztajn JS, Andersen O, Dahllöf I (2012) Lead isotopes in marine surface sediments reveal historical use of leaded fuel. J Environ Monit 14:2893–2901

    Article  CAS  Google Scholar 

  • Lasheen MR, Sharaby CM, El-Kholy NG, Elsherif IY, El-Wakeel ST (2008) Factors influencing lead and iron release from some Egyptian drinking water pipes. J Hazard Mater 160:675–680

    Article  CAS  Google Scholar 

  • Lee RG, Becker WC, Collins DW (1989) Lead at the tap: sources and control. J Am Water Works Assoc 81:52–62

    CAS  Google Scholar 

  • Lyon TDB, Lenihan JMA (1977) Corrosion in solder jointed copper tubes resulting in lead contamination of drinking water. Br Corros J 12:41–45

    Article  CAS  Google Scholar 

  • Lytle DA, Schock MR (1993) Impact of pH and lead composition on metal leached from brass coupons. Environmental Protection Agency Office of Research and Development, Cincinnati

    Google Scholar 

  • Maas RP, Morgan DM, Pandolfo TJ, Patch SC (2005) Reducing lead exposure from drinking water: recent history and current status. Public Health Rep 120:316

    Google Scholar 

  • Magyar M, Ladson A, Diaper C, Mitchell V (2014) Influence of roofing materials and lead flashing on rainwater tank contamination by metals. Aust J Water Resour 18:71–84

    Article  Google Scholar 

  • Murrell NE (1985) Summary of impact of metallic solders on water quality. Water Engineering Research Laboratory Office of Research and Development, Cincinnati

    Google Scholar 

  • Neff CH, Schock MR, Marden JI (1987) Relationships between water quality and corrosion of plumbing materials in buildings. Water Engineering Research Laboratory, Cincinnati

    Google Scholar 

  • Nguyen CK, Stone KR, Dudi A, Edwards MA (2010) Corrosive microenvironments at lead solder surfaces arising from galvanic corrosion with copper pipe. Environ Sci Technol 44:7076–7081

    Article  CAS  Google Scholar 

  • NHMRC (2011) Australian Drinking Water Guidelines Paper 6 National Water Quality Management Strategy. National Health and Medical Research Council. National Resource Management Ministerial Council, Commonwealth of Australia, Canberra

    Google Scholar 

  • O'Byrne M (2013) RE: Correspondene regarding Pioneer drinking water supply, 11 March 2013. Personal communication to LUCK, C

  • Rajaratnam G, Winder C, An M (2002) Metals in drinking water from new housing estates in the Sydney area. Environ Res 89:165–170

    Article  CAS  Google Scholar 

  • Schock MR, Neff CH (1988) Trace metal contamination from brass fittings. J Am Water Works Assoc 80:47–56

    CAS  Google Scholar 

  • Smith C (1992) Moorina power development. Sixth National Conference on Engineering Heritage, 1992. Hobart 5-7 October 1992

  • Subramanian KS, Connor JW (1991) Lead contamination of drinking water. J Environ Health 54:29–32

    CAS  Google Scholar 

  • TASWATER (2013) Quarterly chemical testing—Pioneer 2010–2013. Taswater, Northern Region

    Google Scholar 

  • TASWATER. (2014) Winnaleah boil water alert [online]. http://www.taswater.com.au/Current-Alerts/Boil-Water-Alerts/Winnaleah-Boil-Water-Alert. Accessed 20 Apr 2014

  • Townsend A, Yu Z, Mcgoldrick P, Hutton JA (1998) Precise lead isotope ratios in Australian galena samples by high resolution inductively coupled plasma mass spectrometry. J Anal At Spectrom 13:809–813

    Article  CAS  Google Scholar 

  • Triantafyllidou S, Edwards M (2011) Lead (Pb) in tap water and in blood: implications for lead exposure in the United States. Crit Rev Environ Sci Technol 42:1297–1352

    Article  Google Scholar 

  • UNDG (United Nations Development Goal) (2010) MDG good practice chapter 4 MDG-7 environmental sustainability. United Nations Development Group

  • WHO (World Health Organisation) (1973) Health aspects relating to the use of UPVC pipes for community water supply: a report of a consultant group. WHO International Reference Centre for Community Water Supply

  • WHO (World Health Organisation) (2012) Progress on drinking water and sanitation. World Health Organisation and UNICEF, United States of America

    Google Scholar 

  • WHO (World Health Organisation) (2013) Water quality and health strategy 2013–2020. World Health Organisation

  • Zietz B, Dassel de Vergara J, Kevekordes S, Dunkelberg H (2001) Lead contamination in tap water of households with children in Lower Saxony, Germany. Sci Total Environ 275:19–26

    Article  CAS  Google Scholar 

Download references

Acknowledgments

Thank you to Jenny Bellinger and Lin Simpson for all their help in Pioneer. Thank you to the numerous fieldwork assistants. Peter Weiland of Macquarie University, Michael Wu and Andrew Evans of the Inorganics Laboratory at the National Measurement Institute are thanked for laboratory assistance. This project was funded by a Macquarie University Research Excellence Scholarship (MQRES) (2012195) associated with an Australian Research Council Future Fellowship (FT120100440).

Ethics statement

The Australian National Health and Medical Research Council National Statement of Ethical Conduct in Human Research does not require ethics approval for collection of environmental samples (including tap water, soils or dust) as they do not relate specifically to human health, medicine and human research. Informed consent was however sought from all participants who provided a water sample in this study. Animals were not used in this study.

Conflict of interest

The authors declare no conflict of interest.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to P. J. Harvey.

Additional information

Responsible editor: Philippe Garrigues

Electronic supplementary material

Below is the link to the electronic supplementary material.

ESM 1

(PDF 439 kb)

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Harvey, P.J., Handley, H.K. & Taylor, M.P. Identification of the sources of metal (lead) contamination in drinking waters in north-eastern Tasmania using lead isotopic compositions.. Environ Sci Pollut Res 22, 12276–12288 (2015). https://doi.org/10.1007/s11356-015-4349-2

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11356-015-4349-2

Keywords