Abstract
This study utilises a range of scientific approaches, including lead isotopic compositions, to differentiate unknown sources of ongoing lead contamination of a drinking water supply in north-eastern Tasmania, Australia. Drinking water lead concentrations are elevated above the Australian Drinking Water Guideline (10 μg/L), reaching 540 μg/L in the supply network. Water lead isotopic compositions from the town of Pioneer (208Pb/207Pb 2.406, 206Pb/207Pb 1.144 to 208Pb/207Pb 2.360, 206Pb/207Pb 1.094) and Ringarooma (208Pb/207Pb 2.398, 206Pb/207Pb 1.117) are markedly different from the local bedrock (208Pb/207Pb 2.496, 206Pb/207Pb 1.237). The data show that the lead in the local waters is sourced from a combination of dilapidated drinking water infrastructure, including lead jointed pipelines, end-of-life polyvinyl chloride pipes and household plumbing. Drinking water is being inadvertently contaminated by aging infrastructure, and it is an issue that warrants investigation to limit the burden of disease from lead exposure.






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ABS (Australian Bureau of Statistics) (2011) Census of population and housing basic community profile [online]. Available: http://www.censusdata.abs.gov.au/census_services/getproduct/census/2011/communityprofile/GL_TAS502?opendocument&navpos=230. Accessed 26 Sep 2014
Al-Malack MH (2001) Migration of lead from unplasticized polyvinyl chloride pipes. J Hazard Mater 82:263–274
Balazs C, Ray I (2014) The drinking water disparities framework: on the origins and persistence of inequalities in exposure. Am J Public Health 104:603–611
Beswick A (2012) Pioneer interurption to water supply—community information. Ben Lomond Water, Launceston
Black LP, Everard JL, Mcclenaghan MP, Korsch RJ, Calver CR, Fioretti AM, Brown AV, Foudoulis C (2010) Controls on Devonian-Carboniferous magmatism in Tasmania, based on inherited zircon age patterns, Sr, Nd and Pb isotopes, and major and trace element geochemistry. Aust J Earth Sci 57:933–968
Cirarda FB (1998) Lead in drinking water in the Greater Bilbao Area (Basque Country, Spain). Food Addit Contam 15:575–579
Debenham AJ (1910) Frome Dam, Moorina, Tasmania. Paper read before the Sydney University Engineering Society
del Toral MA, Porter A, Schock MR (2013) Detection and evaluation of elevated lead release from service lines: a field study. Environ Sci Technol 47:9300–9307
DHHS (Tasmanian Department of Health and Human Services) (2014a) Royal george water quality update [online]. Department of Health and Human Services. Available: http://www.dhhs.tas.gov.au/peh/alerts/public_health_updates/royal_george. Accessed 15 May 2014
DHHS (Tasmanian Department of Health and Human Services) (2014b) Rosebery water alert [online]. Department of Health and Human Services. Available: http://www.dhhs.tas.gov.au/news/2013/rosebery_water_alert. Accessed 15 May 2014
Dickens DJ (1990) The Mount Cameron Water Race a century of operation [online]. Tasmanian Department of Resources and Energy. Division of Mines and Mineral Resources - Report 1990/15. http://www.mrt.tas.gov.au/mrtdoc/dominfo/download/UR1990_15/UR1990_15.pdf. Accessed 19 March 2015
Englert N, Höring H (1994) Lead concentration in tap-water and in blood of selected schoolchildren in Southern Saxonia. Toxicol Lett 72:325–331
Evans A (2013) National Measurement Institute, Inorganics Section, Method NT2.63: Determination of isotopic ratios in water and aqueous extracts by high resolution inductively coupled plasma mass spectometry. National Measurement Institute, Australian Government, North Ryde
GHD (GHD Group) (2013a) Report for Ben Lomond Water—BLW drinking water quality options for small towns, 32/16667. Hobart
GHD (GHD Group) (2013b) Report for Ben Lomond Water—Winnaleah, Herrick, Pioneer and Gladstone full treatment water supply options, 32/10294. Hobart
Graham CMW, Andrew B, Gilmour WH, Michael RM, Gordon DM, Stuart JR, John W (1996) Is lead in tap water still a public health problem? An observational study in Glasgow. Br Med J 313:979
Gulson BL (1985) Shale-hosted lead-zinc deposits in northern Australia; lead isotope variations. Econ Geol 80:2001–2012
Gulson BL (1986) Lead isotopes in mineral exploration. Elsevier, USA
Gulson BL, Law AJ, Korsch MJ, Mizon KJ (1994) Effect of plumbing systems on lead content of drinking water and contribution to lead body burden. Sci Total Environ 144:279–284
Harvey PJ, Taylor MP, Handley HK (In review) Widespread environmental contamination hazards in agricultural soils from the use of lead joints in above ground large-scale water supply pipelines. Water Air and Soil Pollution
Heathcote M (2009) History of plastic pipe systems in Australia—general technical information. Plastics Industry Pipe Association of Australia Limited
Hergt J, Chappell B, Mcculloch M, Mcdougall I, Chivas R (1989) Geochemical and isotopic constraints on the origin of the Jurassic Dolerites of Tasmania. J Petrol 30:840–883
Jane Wyatt C, Fimbres C, Romo L, Méndez RO, Grijalva M (1998) Incidence of heavy metal contamination in water supplies in Northern Mexico. Environ Res 76:114–119
Jaquet JB (1894) Geology of the Broken Hill Lode and Barrier Ranges Mineral Field, New South Wales. Department of Mines and Agriculture, Sydney
Johri M, Chandra D, Subramanian SV, Sylvestre M-P, Pahwa S (2014) MDG 7c for safe drinking water in India: an illusive achievement. Lancet 383:1379
Knighton AD (1987) Tin mining and sediment supply to the Ringarooma River, Tasmania, 1875–1979. Aust Geogr Stud 25:83–97
Knighton AD (1989) River adjustment to changes in sediment load: the effects of tin mining on the Ringarooma River, Tasmania, 1875–1984. Earth Surf Process Landf 14:333–359
Knighton AD (1991) Channel bed adjustment along mine-affected rivers of northeast Tasmania. Geomorphology 4:205–219
Knighton AD (1999) The gravel–sand transition in a disturbed catchment. Geomorphology 27:325–341
Kristensen L, Taylor M, Morrison A (2015) Lead and zinc dust depositions from ore trains chracterised using lead isotopic compositions. Environ Sci Processes Impacts 17:631–637
Kristensen L, Taylor M, Odigie K, Hibdon S, Flegal A (2014) Lead isotopic compositions of ash sourced from Australian bushfires. Environ Pollut 190:159–165
Lanphear B, Dietrich K, Auinger P, Cox C (2000) Cognitive deficits associated with blood lead concentrations <10 microg/dL in US children and adolescents. Environ Health Perspect 115:521–529
Lanphear B, Hornung R, Khoury J, Yolton K, Baghurst P, Bellinger D, Canfield R, Dietrich K, Bornschein R, Greene T, Rothenberg S, Needleman H, Schnass L, Wasserman L, Graziano J, Roberts R (2005) Low-level environmental lead exposure and children’s intellectual function: an international pooled analysis. Environ Health Perspect 113:894–899
Larsen MM, Blusztajn JS, Andersen O, Dahllöf I (2012) Lead isotopes in marine surface sediments reveal historical use of leaded fuel. J Environ Monit 14:2893–2901
Lasheen MR, Sharaby CM, El-Kholy NG, Elsherif IY, El-Wakeel ST (2008) Factors influencing lead and iron release from some Egyptian drinking water pipes. J Hazard Mater 160:675–680
Lee RG, Becker WC, Collins DW (1989) Lead at the tap: sources and control. J Am Water Works Assoc 81:52–62
Lyon TDB, Lenihan JMA (1977) Corrosion in solder jointed copper tubes resulting in lead contamination of drinking water. Br Corros J 12:41–45
Lytle DA, Schock MR (1993) Impact of pH and lead composition on metal leached from brass coupons. Environmental Protection Agency Office of Research and Development, Cincinnati
Maas RP, Morgan DM, Pandolfo TJ, Patch SC (2005) Reducing lead exposure from drinking water: recent history and current status. Public Health Rep 120:316
Magyar M, Ladson A, Diaper C, Mitchell V (2014) Influence of roofing materials and lead flashing on rainwater tank contamination by metals. Aust J Water Resour 18:71–84
Murrell NE (1985) Summary of impact of metallic solders on water quality. Water Engineering Research Laboratory Office of Research and Development, Cincinnati
Neff CH, Schock MR, Marden JI (1987) Relationships between water quality and corrosion of plumbing materials in buildings. Water Engineering Research Laboratory, Cincinnati
Nguyen CK, Stone KR, Dudi A, Edwards MA (2010) Corrosive microenvironments at lead solder surfaces arising from galvanic corrosion with copper pipe. Environ Sci Technol 44:7076–7081
NHMRC (2011) Australian Drinking Water Guidelines Paper 6 National Water Quality Management Strategy. National Health and Medical Research Council. National Resource Management Ministerial Council, Commonwealth of Australia, Canberra
O'Byrne M (2013) RE: Correspondene regarding Pioneer drinking water supply, 11 March 2013. Personal communication to LUCK, C
Rajaratnam G, Winder C, An M (2002) Metals in drinking water from new housing estates in the Sydney area. Environ Res 89:165–170
Schock MR, Neff CH (1988) Trace metal contamination from brass fittings. J Am Water Works Assoc 80:47–56
Smith C (1992) Moorina power development. Sixth National Conference on Engineering Heritage, 1992. Hobart 5-7 October 1992
Subramanian KS, Connor JW (1991) Lead contamination of drinking water. J Environ Health 54:29–32
TASWATER (2013) Quarterly chemical testing—Pioneer 2010–2013. Taswater, Northern Region
TASWATER. (2014) Winnaleah boil water alert [online]. http://www.taswater.com.au/Current-Alerts/Boil-Water-Alerts/Winnaleah-Boil-Water-Alert. Accessed 20 Apr 2014
Townsend A, Yu Z, Mcgoldrick P, Hutton JA (1998) Precise lead isotope ratios in Australian galena samples by high resolution inductively coupled plasma mass spectrometry. J Anal At Spectrom 13:809–813
Triantafyllidou S, Edwards M (2011) Lead (Pb) in tap water and in blood: implications for lead exposure in the United States. Crit Rev Environ Sci Technol 42:1297–1352
UNDG (United Nations Development Goal) (2010) MDG good practice chapter 4 MDG-7 environmental sustainability. United Nations Development Group
WHO (World Health Organisation) (1973) Health aspects relating to the use of UPVC pipes for community water supply: a report of a consultant group. WHO International Reference Centre for Community Water Supply
WHO (World Health Organisation) (2012) Progress on drinking water and sanitation. World Health Organisation and UNICEF, United States of America
WHO (World Health Organisation) (2013) Water quality and health strategy 2013–2020. World Health Organisation
Zietz B, Dassel de Vergara J, Kevekordes S, Dunkelberg H (2001) Lead contamination in tap water of households with children in Lower Saxony, Germany. Sci Total Environ 275:19–26
Acknowledgments
Thank you to Jenny Bellinger and Lin Simpson for all their help in Pioneer. Thank you to the numerous fieldwork assistants. Peter Weiland of Macquarie University, Michael Wu and Andrew Evans of the Inorganics Laboratory at the National Measurement Institute are thanked for laboratory assistance. This project was funded by a Macquarie University Research Excellence Scholarship (MQRES) (2012195) associated with an Australian Research Council Future Fellowship (FT120100440).
Ethics statement
The Australian National Health and Medical Research Council National Statement of Ethical Conduct in Human Research does not require ethics approval for collection of environmental samples (including tap water, soils or dust) as they do not relate specifically to human health, medicine and human research. Informed consent was however sought from all participants who provided a water sample in this study. Animals were not used in this study.
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Harvey, P.J., Handley, H.K. & Taylor, M.P. Identification of the sources of metal (lead) contamination in drinking waters in north-eastern Tasmania using lead isotopic compositions.. Environ Sci Pollut Res 22, 12276–12288 (2015). https://doi.org/10.1007/s11356-015-4349-2
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DOI: https://doi.org/10.1007/s11356-015-4349-2